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研究生： 陳梅儂
Mei-Nung Chen
論文名稱： 共軛高分子提升載子遷移率暨光誘導可恢復機制在有機場效應電晶體的探討
Conjugated Polymers for the Mobility Boosting and the Photoinduced Recovery Mechanism in OFET
指導教授： 邱昱誠
Yu-Cheng Chiu
口試委員: 邱昱誠
Yu-Cheng Chiu
江偉宏
Wei-Hung Chiang
王建隆
Chien-Lung, Wang
學位類別： 碩士
Master
系所名稱： 工程學院 - 化學工程系
Department of Chemical Engineering
論文出版年： 2021
畢業學年度： 109
語文別： 中文
論文頁數： 137
中文關鍵詞： 有機場效應電晶體 、共軛高分子 、混參系統半導體 、載子遷移率提升 、光誘導可恢復機制
外文關鍵詞： Organic Field-Effect Transistor, Conjugated Polymer, Blend System Semiconductor, Mobility Booster, Photoinduced Recovery Mechanism
相關次數： 點閱：225  下載：0 
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    • Table of Content 致謝 I ABSTRACT II 中文摘要 IV CHAPTER 1 16 1.2. ORGANIC FIELD-EFFECT TRANSISTORS (OFETS) 16 1.2.1. OFET Device Structure and principle 16 1.2.2. Charge-Carrier Mobility 17 1.2.3. Organic Semiconductor Materials for OFETs 20 1.3. SEMICONDUCTORS FOR HIGH PERFORMANCE OFETS 21 1.3.1. Modifying with Dielectric 22 1.3.2. Contact Resistance 23 1.3.3. Molecular Design Strategies for High-Performance D-A-Conjugated Polymers 23 1.3.3.1. Planar and Rigid Backbone 25 1.3.3.2. Close Intermolecular Packing 26 1.3.3.3. Molecular Weight 27 1.3.3.4. Molecular Design Strategies for High-Performance D-A Conjugated Polymers 27 1.4. THE MULTICOMPONENT OSC SYSTEMS OF THE OFET DEVICE TO IMPROVE THE MOBILITY 29 1.4.1 Doped Organic Transistors 30 1.4.2. Organic Semiconductor/Polymer Blending Films 34 1.4.2.1. Small-Molecule Semiconductor/Insulating Polymer Blend System 35 1.4.2.2. Small-Molecule Semiconductor/Conjugated Polymer Blend System 37 1.4.2.3. Polymer Semiconductor/Insulating Polymer Blend System 37 1.4.2.4. Polymer Semiconductor/Conjugated Polymer Blend System 44 1.5. OFET-BASED NONVOLATILE MEMORY DEVICES 45 1.5.1. Operation principle of OFET memory devices 47 1.5.2. Polymer electrets for non-volatile memory devices 50 1.5.3. Non-Volatile Photonic Memory 51 1.5.3.1 Semiconductor Effect on Photo-Induced Recovery Phenomena 51 1.5.3.2 Floating-Gate Effect on Photo-Induced Recovery Phenomena 54 1.5.3.3 Polymer Electret Effect on Photo-Induced Recovery Phenomena 56 1.6 RESEARCH MOTIVATION 61 CHAPTER 2 63 ABSTRACT 63 2.1. INTRODUCTION 64 2.2. EXPERIMENTAL SECTION 67 2.2.1. Materials 67 2.2.2. Device Fabrication and Device Structure 68 2.2.3. Characterization 68 2.3. RESULTS AND DISCUSSION 68 2.3.1 The performance of PDPP-TVT/PTPA-3CN blend system 68 2.3.2. The Annealing Condition of PDPP-TVT/PTPA-3CN Blend System 77 2.3.3. The Influence of Molecular-Design Strategy of Additives Blended into Conjugated Polymer 79 2.4 CONCLUSION 87 CHAPTER 3 89 ABSTRACT 89 3.1. INTRODUCTION 90 3.2. EXPERIMENTAL SECTION 92 3.2.1. Materials 92 3.2.2. Device Fabrication and Device Structure 93 3.2.3. Characterization 93 3.3. RESULTS AND DISCUSSION 94 3.3.1. P-Type OFET Memory Employing PFO Polymer as Electret 94 3.3.2. Working Mechanism of Photoinduced Recovery Behavior 103 3.3.3. The Commercial Polymer as Electret for P-Type OFET Memory 105 3.3.4. The Photo-Recorder for PFO Based Electret Memory Devices 107 3.4. CONCLUSION 113 CHAPTER 4 115 Conclusion 115 REFERENCES 117 Chapter 1 117 Chapter 2 124 Chapter 3 127

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    Chapter 2
    1. Horowitz, G., Organic Field-Effect Transistors. Adv. Mater. 1998, 10, 365-377.
    2. Guo, Y.; Yu, G.; Liu, Y., Functional organic field-effect transistors. Adv. Mater. 2010, 22 (40), 4427-47.
    3. Dong, H.; Fu, X.; Liu, J.; Wang, Z.; Hu, W., 25th anniversary article: key points for high-mobility organic field-effect transistors. Adv Mater 2013, 25 (43), 6158-83.
    4. Shih, C. C.; Chiang, Y. C.; Hsieh, H. C.; Lin, Y. C.; Chen, W. C., Multilevel Photonic Transistor Memory Devices Using Conjugated/Insulated Polymer Blend Electrets. ACS Appl. Mater. Interfaces 2019, 11 (45), 42429-42437.
    5. Chiang, Y. C.; Hung, C. C.; Lin, Y. C.; Chiu, Y. C.; Isono, T.; Satoh, T.; Chen, W. C., High-Performance Nonvolatile Organic Photonic Transistor Memory Devices using Conjugated Rod-Coil Materials as a Floating Gate. Adv. Mater. 2020, 32 (36), e2002638.
    6. Kim, M.; Ryu, S. U.; Park, S. A.; Choi, K.; Kim, T.; Chung, D.; Park, T., Donor–Acceptor‐Conjugated Polymer for High‐Performance Organic Field‐Effect Transistors: A Progress Report. Adv. Funct. Mater. 2019, 30 (20).
    7. Yu, H.; Park, K. H.; Song, I.; Kim, M.-J.; Kim, Y.-H.; Oh, J. H., Effect of the alkyl spacer length on the electrical performance of diketopyrrolopyrrole-thiophene vinylene thiophene polymer semiconductors. Journal of Materials Chemistry C 2015, 3 (44), 11697-11704.
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    11. Ocheje, M. U.; Charron, B. P.; Cheng, Y. H.; Chuang, C. H.; Soldera, A.; Chiu, Y. C.; Rondeau-Gagné, S., Amide-Containing Alkyl Chains in Conjugated Polymers: Effect on Self-Assembly and Electronic Properties. Macromolecules 2018, 51 (4), 1336-1344.
    12. Kim, J. H.; Yun, S. W.; An, B. K.; Han, Y. D.; Yoon, S. J.; Joo, J.; Park, S. Y., Remarkable mobility increase and threshold voltage reduction in organic field-effect transistors by overlaying discontinuous nano-patches of charge-transfer doping layer on top of semiconducting film. Adv. Mater. 2013, 25 (5), 719-24.
    13. Pan, Y.; Yu, G., Multicomponent Blend Systems Used in Organic Field-Effect Transistors: Charge Transport Properties, Large-Area Preparation, and Functional Devices. Chemistry of Materials 2021, 33 (7), 2229-2257.
    14. Chen, J.; Shao, M.; Xiao, K.; He, Z.; Li, D.; Lokitz, B. S.; Hensley, D. K.; Kilbey, S. M.; Anthony, J. E.; Keum, J. K.; Rondinone, A. J.; Lee, W.-Y.; Hong, S.; Bao, Z., Conjugated Polymer-Mediated Polymorphism of a High Performance, Small-Molecule Organic Semiconductor with Tuned Intermolecular Interactions, Enhanced Long-Range Order, and Charge Transport. Chemistry of Materials 2013, 25 (21), 4378-4386.
    15. Lei, Y.; Deng, P.; Lin, M.; Zheng, X.; Zhu, F.; Ong, B. S., Enhancing Crystalline Structural Orders of Polymer Semiconductors for Efficient Charge Transport via Polymer-Matrix-Mediated Molecular Self-Assembly. Adv. Mater. 2016, 28 (31), 6687-94.
    16. Angunawela, I.; Nahid, M. M.; Ghasemi, M.; Amassian, A.; Ade, H.; Gadisa, A., The Critical Role of Materials' Interaction in Realizing Organic Field-Effect Transistors Via High-Dilution Blending with Insulating Polymers. ACS Appl. Mater. Interfaces 2020, 12 (23), 26239-26249.
    17. Ke, C. Y.; Chen, M. N.; Chiu, Y. C.; Liou, G. S., Luminescence Behavior and Acceptor Effects of Ambipolar Polymeric Electret on Photorecoverable Organic Field‐Effect Transistor Memory. Adv. Electron. Mater. 2021, 7 (3), 2001076.
    18. Zhang, S.; Cheng, Y. H.; Galuska, L.; Roy, A.; Lorenz, M.; Chen, B.; Luo, S.; Li, Y. T.; Hung, C. C.; Qian, Z.; St. Onge, P. B. J.; Mason, G. T.; Cowen, L.; Zhou, D.; Nazarenko, S. I.; Storey, R. F.; Schroeder, B. C.; Rondeau‐Gagné, S.; Chiu, Y. C.; Gu, X., Tacky Elastomers to Enable Tear‐Resistant and Autonomous Self‐Healing Semiconductor Composites. Adv. Funct. Mater. 2020, 30 (27).
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    20. Agostinelli, T.; Lilliu, S.; Labram, J. G.; Campoy-Quiles, M.; Hampton, M.; Pires, E.; Rawle, J.; Bikondoa, O.; Bradley, D. D. C.; Anthopoulos, T. D.; Nelson, J.; Macdonald, J. E., Real-Time Investigation of Crystallization and Phase-Segregation Dynamics in P3HT:PCBM Solar Cells During Thermal Annealing. Adv. Funct. Mater. 2011, 21 (9), 1701-1708.

    Chapter 3
    1. Zhai, Y.; Yang, J. Q.; Zhou, Y.; Mao, J. Y.; Ren, Y.; Roy, V. A. L.; Han, S. T., Toward non-volatile photonic memory: concept, material and design. Mater. Horiz. 2018, 5 (4), 641-654.
    2. Shih, C. C.; Chiang, Y. C.; Hsieh, H. C.; Lin, Y. C.; Chen, W. C., Multilevel Photonic Transistor Memory Devices Using Conjugated/Insulated Polymer Blend Electrets. ACS Appl. Mater. Interfaces 2019, 11 (45), 42429-42437.
    3. Hu, L.; Yuan, J.; Ren, Y.; Wang, Y.; Yang, J. Q.; Zhou, Y.; Zeng, Y. J.; Han, S. T.; Ruan, S., Phosphorene/ZnO Nano-Heterojunctions for Broadband Photonic Nonvolatile Memory Applications. Adv. Mater. 2018, 30 (30), 1801232.
    4. Chen, J. Y.; Chiu, Y. C.; Li, Y. T.; Chueh, C. C.; Chen, W. C., Nonvolatile Perovskite-Based Photomemory with a Multilevel Memory Behavior. Adv. Mater. 2017, 29 (33), 1702217.
    5. Jeong, Y. J.; Yun, D. J.; Kim, S. H.; Jang, J.; Park, C. E., Photoinduced Recovery of Organic Transistor Memories with Photoactive Floating-Gate Interlayers. ACS Appl. Mater. Interfaces 2017, 9 (13), 11759-11769.
    6. Jeong, Y. J.; Yun, D. J.; Noh, S. H.; Park, C. E.; Jang, J., Surface Modification of CdSe Quantum-Dot Floating Gates for Advancing Light-Erasable Organic Field-Effect Transistor Memories. ACS Nano 2018, 12 (8), 7701-7709.
    7. Chen, C. H.; Wang, Y.; Tatsumi, H.; Michinobu, T.; Chang, S. W.; Chiu, Y. C.; Liou, G. S., Novel Photoinduced Recovery of OFET Memories Based on Ambipolar Polymer Electret for Photorecorder Application. Adv. Funct. Mater. 2019, 29 (40), 1902991.
    8. Chen, C. H.; Wang, Y.; Michinobu, T.; Chang, S. W.; Chiu, Y. C.; Ke, C. Y.; Liou, G. S., Donor-Acceptor Effect of Carbazole-Based Conjugated Polymer Electrets on Photoresponsive Flash Organic Field-Effect Transistor Memories. ACS Appl. Mater. Interfaces 2020, 12 (5), 6144-6150.
    9. Ke, C. Y.; Chen, M. N.; Chiu, Y. C.; Liou, G. S., Luminescence Behavior and Acceptor Effects of Ambipolar Polymeric Electret on Photorecoverable Organic Field‐Effect Transistor Memory. Adv. Electron. Mater. 2021, 7 (3), 2001076.
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